气候变化研究进展 ›› 2008, Vol. 4 ›› Issue (004): 195-201.

• 研究论文 •    下一篇

1994-2006年长江三角洲和东北平原酸性气体浓度变化

徐晓斌,林伟立,颜鹏,张忠华,俞向明   

  1. 中国气象科学研究院
  • 收稿日期:2007-10-25 修回日期:2008-01-18 出版日期:2008-07-31 发布日期:2008-07-31
  • 通讯作者: 徐晓斌

Long-term Changes of Acidic Gases in China's Yangtze Delta and Northeast Plain Regions During 1994-2006

Weili Lin,Zhonghua Zhang,Xiangming Yu   

  1. 1. Key Laboratory for Atmospheric Chemistry of China Meteorological Administration, Centre for Atmosphere Watch and Services of China Meteorological Administration, Chinese Academy of Meteorological Scie2. Chinese Academy of Meteorological Sciences
  • Received:2007-10-25 Revised:2008-01-18 Online:2008-07-31 Published:2008-07-31

摘要: 利用长江三角洲和东北平原地区大气本底站的二氧化硫(SO2)和氮氧化物(NOx)历史资料和近期取得的观测数据,探讨两个地区人为排放对这些气候相关酸性气体的不同贡献。从两种酸性气体过去和现在的浓度水平,估算了它们在两个地区的增长率,比较了NOx与SO2比值的不同变化趋势。结果表明,早在20世纪90年代中期,长江三角洲酸性气体污染水平已经较高,其后主要是NOx浓度显著升高,从而使该地区成为硫和氮污染并重的地区;东北平原酸性气体过去浓度很低,但这些气体以很高的速率增长,虽然目前浓度水平仍然比较低,但未来形势不容乐观。

关键词: 气候相关酸性气体, 二氧化硫, 氮氧化物, 人为排放, 东北平原

Abstract: Historic and recent observational data of SO2 and NOx from Lin誥n and Longfengshan background stations, located in the Yangtze Delta and the Northeast Plain region, respectively, are analyzed in order to study the differences in concentrations of these climate-relevant acidic gases between the two regions, and the impacts of anthropogenic emissions on the gases since about one decade ago. The past and more recent concentration levels of the gases are compared between the two sites, long-term changing trends of the gases at both sites are estimated, and the NOx/SO2 ratios for the two sites are obtained using the correlation method. The results show that as early as middle 1990s, concentration levels of SO2 and NOx have been considerably high already at the background station of the Yangtze Delta region, and since then anthropogenic emissions have caused a significant increase in NOx concentration, making NOx another major pollutant in addition to SO2. Data from Longfengshan station suggest that levels of acidic gases in the Northeast Plain region were originally very low in the past, and are still considerably low at present. However, levels of the two acidic gases in this less polluted region have increased at very high rates, therefore, the future levels of these gases in the region are not optimistic.

Key words: climate-relevant acidic gases, sulfur dioxide, nitrogen oxides, anthropogenic emission, Yangtze Delta, Northeast Plain

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